Behavior of disperse media based on magnetic fluids in inhomogeneous magnetic fields
https://doi.org/10.21869/2223-1528-2025-15-1-177-193
Abstract
Purpose. To study the behavior of dispersed media based on nanodispersed magnetic fluids: non-magnetic liquid and gaseous inclusions in a magnetic fluid, drops of magnetic fluid in a non-magnetic medium, as well as non-magnetic bubbles and drops covered with a shell of magnetic fluid in non-uniform magnetic fields.
Methods. The results were obtained experimentally using generally accepted methods and approaches. The setups used for the studies were developed independently, and data were collected using standard measuring equipment. The magnetic field induction value was measured using a TPU-01 teslameter with a Hall transducer connected to it. The magnetic field topology was modeled using the FEMM software embedded in the MathLab interactive environment. The platform not only models the magnetic field, but also qualitatively transforms the calculation results and visualizes them. The images of non-magnetic inclusions were processed in a specially developed program in the NI Labview system. Theoretical processing of the experimental results was based on known expressions of condensed matter physics, magnetic and classical hydrodynamics.
Results. Experimental dependences of the coordinate, velocity, size of dispersed media based on magnetic fluid on the magnetic field parameters, physical properties of magnetic and non-magnetic fluids are obtained. Based on the results of computer modeling in the FEMM program, an assessment of the forces acting on a non-magnetic drop and bubble in a magnetic fluid is carried out. The obtained experimental and theoretical data are consistent with each other.Experimental dependences of the position, velocity, and size of magnetic fluid-based disperse media on magnetic field parameters and the physical properties of magnetic and non-magnetic liquids were obtained. Computer simulations were used to estimate the forces acting on non-magnetic droplets and bubbles in a magnetic fluid. The experimental and theoretical data are in good agreement.
Conclusion. An inhomogeneous magnetic field allows for the control of the dynamics and behavior of magnetic fluidbased disperse media, paving the way for the development of controllable dispensers and systems for synthesizing active droplets.
About the Authors
E. А. SokolovRussian Federation
Evgeniy A. Sokolov, Lecturer of the Department of Nanotechnology, Microelectronics, General and Applied Physics
Kursk
P. A. Riapolov
Petr A. Riapolov, Doctor of Sciences (Physics and Mathematics), Associate Professor, Dean of the Faculty of Natural Science
Kursk
References
1. Rosensweig R.E. Ferrohydrodynamics. Moscow: Mir; 1989. 356 p. (In Russ.)
2. Joseph A., Mathew S. Ferrofluids: synthetic strategies, stabilization, physicochemical features, characterization, and applications. ChemPlusChem. 2014;79(10):1382-1420.
3. Genc S., Derin B. Synthesis and rheology of ferrofluids: a review. Current Opinion in Chemical Engineering. 2014;3:118–124.
4. Papell S.S. Low viscosity magnetic fluid obtained by the colloidal suspension of magnetic particles. United States patent US 3215572A. 2 November 1965.
5. Odenbach S., Gilly H. Taylor vortex flow of magnetic fluids under the influence of an azimuthal magnetic field. Journal of magnetism and magnetic materials. 1996;152(1-2):123–128.
6. Erin K.V., Porublev A.A. Optical properties of kerosene-based magnetic fluids. In: Fizikokhimicheskie i prikladnye problemy magnitnykh dispersnykh nanosistem: V Vserossiiskaya nauchnaya konferentsiya: sbornik nauchnykh trudov = Physico-chemical and applied problems of magnetic dispersed nanosystems: V All-Russian scientific conference: collection of scientific papers. Stavropol': Fabula; 2015. P. 79-85. (In Russ.)
7. Yang X., Dou X., Liu Y., Huang Y. Sealing mechanism investigation of convergent ferrofluid seals with staggered pole teeth. Tribology International. 2023;190:109054. https://doi.org/10.1016/j.triboint.2023.10905.
8. Gao Q.H., Peng Z.Z., Zou H.-X., Li W.B., Yan H., Peng Z., et al. Label-free manipulation via the magneto-Archimedes effect: fundamentals, metho-dology and applications. Materials Horizons. 2019;6(7):1359-1379. https://doi.org/10.1063/1.4867964.
9. Lee C.P., Lan T.S., Lai M.F. Fabrication of two-dimensional ferrofluid microdroplet lattices in a microfluidic channel. Journal of Applied Physics. 2014;115(17):17В527. https://doi.org/10.1063/1.4867964.
10. Bohara R.A., Thorat ND., Pawar S. H. Role of functionalization: Strategies to explore potential nano-bio applications of magnetic nanoparticles. RSC advances. 2016;6(50):43989-44012.
11. Ivanov A.O., Kuznetsova O.B. Magnetic properties of dense ferrofluids: An influence of interparticle correlations. Physical Review E. 2001;64(4):041405.
12. Koskov M.A., Lebedev A.V., Ivanov A.S. On the differential sweep method for obtaining magnetization curves of ferrofluids. Izvestiya Yugo-Zapadnogo gosudarstvennogo universiteta. Seriya: Tekhnika i tekhnologii = Proceedings of the Southwest State University. Series: Engineering and Technology. 2023;13(3):89-104. (In Russ.) https://doi.org/10.21869/2223-1528-2023-13-3-89-104.
13. Hewlin Jr R.L., Edwards M., Schultz C. Design and development of a traveling wave ferromicrofluidic device and system rig for potential magnetophoretic cell separation and sorting in a waterbased ferrofluid. Micromachines. 2023;14(4):889.
14. Brown P., Hatton T.A., Eastoe J. Magnetic surfactants. Current Opinion in Colloid & Interface Science. 2015;20(3):140-150.
15. Huang X., Saadat M., Bijarchi M.A., Shafii M.B. Ferrofluid double emulsion generation and manipulation under magnetic fields. Chemical Engineering Science. 2023;270:118519.
16. Bashtovoi V., Kovalev M., Reks A. Instabilities of bubbles and droplets flows in magnetic fluids. Journal of magnetism and magnetic materials. 2005;289:350-352.
17. Sokolov E.A., Kalyuzhnaya D.A., Reks A.G., Kalenchuk V.I., Zhukov G.A., Politov R.E., et al. Dynamics of active bubbles in a magnetic fluid in an inhomogeneous magnetic field. Izvestiya YugoZapadnogo gosudarstvennogo universiteta. Seriya: Tekhnika i tekhnologii = Proceedings of the Southwest State University. Series: Engineering and Technology. 2023;13(1):102-119. (In Russ.) https://doi.org/10.21869/2223-1528-2023-13-1-102-119.
18. Pohl H.A. Some effects of nonuniform fields on dielectrics. Journal of Applied Physics. 1958; 29(8):1182–1188.
19. Srinivasan G.J., Satyanarayana P., Thirunavukkarasu G. Liquid drops in rise against gravity through a viscous medium: Drag force by the method of dimensions and comparison with liquid drops in fall under gravity. Current Science. 1996;71(12):989-995.
20. Sokolov E., Kalyuzhnaya D., Ryapolov P. Behavior of non–magnetic liquid-magnetic fluid» emulsions in microchannels under the influence of an inhomogeneous magnetic field. IEEE Transactions on Magnetics. 2025. URL: https://ieeexplore.ieee.org/document/10900568/. https://doi.org/10.1109/TMAG.2025.3544657.
21. Sokolov E.A., Kalyuzhnaya D.A., Pribylov A.A., Politov R.E., Ryapolov P.A. Dynamics of floating droplets of a magnetic liquid in glycerol in a flat channel under the influence of a magnetic field. Bulletin of the Russian Academy of Sciences: Physics. 2024;88(10):1636-1641.
22. Sokolov E., Kaluzhnaya D., Shel’deshova E., Ryapolov P. Formation and behaviour of active droplets and bubbles in a magnetic fluid in an inhomogeneous magnetic field. Fluids. 2022;8(1):2. https://doi.org/10.3390/fluids8010002.
Review
For citations:
Sokolov E.А., Riapolov P.A. Behavior of disperse media based on magnetic fluids in inhomogeneous magnetic fields. Proceedings of the Southwest State University. Series: Engineering and Technology. 2025;15(1):177-193. (In Russ.) https://doi.org/10.21869/2223-1528-2025-15-1-177-193